By implanting silicon ions in diamond with extreme precision and then controlling the strain on the crystal structure, scientists showed that they could significantly increase the spin lifetimes of solid-state quantum bits. This is of fundamental importance to quantum mechanics and quantum computing.
Quantum networks could change how we produce and send data. Creating such networks requires generating single phonons—the vibrational motion that characterizes single atoms and nonclassical mechanical states. This work opens the door to achieving a long sought-after goal: deterministically producing phonons. These phonons could be used to interface with other quantum systems such as superconducting qubits. The strain engineering approach developed in this research can also be applied to other quantum emitters and be used to generate scalable quantum networks.
Solid-state quantum bits, or qubits, offer scalability in a quantum network. Such networks could change how computations are done and how data is sent. However, the uncontrolled interaction of a quantum system with its environment can cause the quantum states to collapse, a.k.a. quantum decoherence. While there are a range of techniques available to reduce environmental effects, overcoming thermal decoherence is more challenging. Typically, the only effective strategy is to maintain the quantum system at extremely low temperatures. In Nature Communications, a team shows a different approach to solving this problem. They started with the negatively charged silicon-vacancy center in a diamond, an emerging building block for photonic quantum networks. Scientists created these silicon-vacancy centers at the Center for Integrated Nanotechnologies using a focused ion beam to precisely implant silicon ions in an array on a diamond substrate. Normally this type of device would be subject to thermal decoherence unless the quantum system is operated at ultracold temperatures. Instead of lowering the temperature, the team took advantage of the fact that the electron-phonon coupling, which is the cause of the thermal decoherence, arises from a high susceptibility of the electronic orbitals to lattice strain. They devised a way to increase the strain. They achieved this with a nano-electro-mechanical system device—a single-crystal diamond cantilever with metal electrodes patterned above and below it. An opening in the top electrode allows optical access to the silicon-vacancy qubits. A direct current voltage applied across the electrodes deflects the cantilever downwards and generates controllable static strain. Through strain control, the team reduced the electron-phonon coupling and demonstrated six-fold improvement in the spin coherence time.
Center for Integrated Nanotechnologies and Sandia National Laboratories
This work was supported by STC Center for Integrated Quantum Materials (National Science Foundation (NSF)), Office of Naval Research Multidisciplinary University Research Initiatives on Quantum Optomechanics, NSF Emerging Frontiers in Research and Innovation Advancing Communication and Quantum Information Research in Engineering, the University of Cambridge, the European Research Council Consolidator Grant PHOENICS, and the Engineering and Physical Sciences Research Council Quantum Technology Hub Networked Quantum Information Technologies. B.P. thanks Wolfson College (University of Cambridge) for support through a research fellowship. Device fabrication was performed in part at the Center for Nanoscale Systems (CNS), a member of the National Nanotechnology Infrastructure Network, which is supported by NSF. CNS is part of Harvard University. Focused ion beam implantation was performed under the Laboratory Directed Research and Development Program and the Center for Integrated Nanotechnologies, a Department of Energy Office of Science user facility at Sandia National Laboratories.
Y.I. Sohn, S. Meesala, B. Pingault, A.A. Atikian, J. Holzgrafe, M. Gündo?an, C. Stavrakas, M.J. Stanley, A. Sipahigil, J. Choi, M. Zhang, J.L. Pacheco, J. Abraham, E. Bielejec, M.D. Lukin, M. Atatüre, and M. Lon?ar, "Controlling the coherence of a diamond spin qubit through its strain environment." Nature Communications 9, 2012 (2018). [DOI: 10.1038/s41467-018-04340-3]