Atoms in magnetic materials are organized into regions called magnetic domains. Within each domain, the electrons have the same magnetic orientation. This means their spins point in the same direction. “Walls” separate the magnetic domains. One type of wall has spin rotations that are left- or right-handed, known as having chirality. When subjected to a magnetic field, chiral domain walls approach one another, shrinking the magnetic domains. Researchers have developed a magnetic material whose thickness determines whether chiral domain walls have the same or alternating handedness. In the latter case, applying a magnetic field leads to annihilation of colliding domain walls. The researchers combined neutron scattering and electron microscopy to characterize these internal, microscopic features, leading to better understanding of the magnetic behavior.
An emerging field of technology called spintronics involves processing and storing information by harnessing an electron’s spin instead of its charge. The ability to control this fundamental property could unlock new possibilities for developing electronic devices. Compared to current technology, these devices could store more information in less space and operate at higher speeds with less energy consumption. This study demonstrates a way to change the rotational direction and occurrence of domain wall pairs. This suggests a potential route for controlling domain walls’ properties and movement. The results could have implications for technologies based on spintronics.
The ability to manipulate domain wall movement has remained a challenge because typically magnetic domains can randomly switch orientations. In addition, domain boundaries move unpredictably when domain sizes are reduced to accommodate higher information storage density. However, a class of materials called chiral magnets has shown potential for mitigating random domain wall behavior. This is because chiral magnets exhibit intricate spin structures, which help reduce the random reversal of domains.
Researchers from Indiana University–Purdue University Indianapolis, Oak Ridge National Laboratory, Louisiana State University, Norfolk State University, the Peter Grünberg Institute, and the University of Louisiana at Lafayette developed a chiral magnetic material by inserting manganese atoms between hexagonal layers of niobium disulfide compounds. By performing neutron experiments at the High Flux Isotope Reactor (HFIR), the team was able to analyze the magnetic nanostructure of the material when subjected to different temperatures and magnetic fields. These measurements were combined with characterization via Lorentz transmission electron microscopy, allowing a more complete understanding of the magnetic behavior. The team’s data suggest that changing the thickness of the chiral magnet can cause some domain wall pairs to rotate in opposite directions, known as having opposite chirality. Furthermore, the researchers found that domain walls with opposite chirality will move toward each other and annihilate when exposed to an external magnetic field. The findings could inform future research on controlling magnetic properties for technological applications.
Oak Ridge National Laboratory
Indiana University–Purdue University Indianapolis
The research was supported by the Department of Energy (DOE) Established Program to Stimulate Competitive Research, the National Science Foundation, the European Research Council, the German Research Foundation, and the Louisiana Board of Regents. Research was performed at High Flux Isotope Reactor at Oak Ridge National Laboratory, a DOE Office of Science user facility.
Karna, S., et al., Annihilation and Control of Chiral Domain Walls with Magnetic Fields. Nano Letters 21, 3, 1205-1212 (2021). [DOI: 10.1021/acs.nanolett.0c03199]
Magnetic Field Control of Chiral Domain Walls in Mn1/3NbS2, Oak Ridge National Laboratory highlight